You can't query against the DataTable's Rows collection, since DataRowCollection doesn't implement IEnumerable<T>. You need to use the AsEnumerable() extension for DataTable. Like so:

var results = from myRow in myDataTable.AsEnumerable()
where myRow.Field<int>("RowNo") == 1
select myRow;

And as @Keith says, you'll need to add a reference to System.Data.DataSetExtensions

AsEnumerable() returns IEnumerable<DataRow>. If you need to convert IEnumerable<DataRow> to a DataTable, use the CopyToDataTable() extension.

Below is query with Lambda Expression,

var result = myDataTable
    .AsEnumerable()
    .Where(myRow => myRow.Field<int>("RowNo") == 1);